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The Omnic Crisis is very important. It was a global catastrophe that led to the formation of Overwatch. Another is the fall of Overwatch due to internal issues. And the rise of Talon as a major threat is also a key event.
Characterization is also difficult. The characters in Overwatch have their own distinct personalities and backstories, and the same goes for those in Game of Thrones. When bringing them together, you have to make sure their interactions are believable. For instance, Mercy from Overwatch is a healer with a very different moral code compared to some of the morally ambiguous characters in Game of Thrones.
You can start by looking on fanfiction websites like Archive of Our Own (AO3). It has a large collection of Overwatch fanfictions. Another good place is FanFiction.net. There are also Overwatch - related forums where fans might share their own fanfictions or recommend good ones.
To write a good Overwatch fanfiction, start with a strong hook to draw readers in. It could be a mysterious event or a character in a difficult situation. Build on the existing Overwatch universe but add your own twists. For example, explore how a new villain could affect the heroes. And use vivid descriptions to make the story come alive. For instance, when describing a battle, talk about the flash of the guns, the sound of the explosions, and the expressions on the heroes' faces.