One of the Legendary Pokemon could be Giratina. Despite its somewhat dark and otherworldly nature, Giratina might be intrigued by Ash's light - heartedness and his ability to make friends with all kinds of Pokemon. Dialga and Palkia could also be part of the harem. Dialga, with its control over time, might see Ash as an important factor in the future of the Pokemon world. Palkia, in charge of space, could be interested in how Ash navigates different regions and spaces in his journey. And don't forget about Ho - Oh. Ho - Oh is a symbol of hope and might see Ash as a bringer of hope in the Pokemon world, thus joining his harem.
Articuno, Zapdos, and Moltres are quite common. Their elemental powers and the mystery surrounding them make for great fanfiction material. Ash might encounter them during his travels and have to either help them or face off against them in some way.
Arceus is quite popular. Given that it's considered the creator of the Pokemon universe in the official lore, it often has a significant role in fanfictions. Mewtwo is also very common. Its powerful psychic abilities and complex backstory make it a favorite for fanfic writers to explore. Another popular one is Lugia. With its majestic appearance and its connection to the sea, it's often a central figure in many stories.
A great plot might be that Ash accidentally stumbles upon a hidden realm where Legendary Pokemon live in seclusion. His presence disrupts their normal life, but instead of being angry, they are intrigued by this human. Ash shows them his love for Pokemon through his actions. As a result, one by one, the Legendary Pokemon start to follow him around. His harem grows, and with their combined powers and his leadership, they start to take on challenges like saving other Pokemon from a new and dangerous disease that is spreading and is said to be related to an ancient curse that only the Legendaries can help break.
It could be Mew. Mew is known for its ability to transform and has a very mysterious nature. If Ash was Mew's son, he might inherit some of that mystery and the power to communicate with Pokemon in unique ways.
Obviously, Ash is one of the main characters. Since it's about him being a legendary Pokemon in this fanfiction, he's central to the story.
There are also fanfictions where Ash catches Rayquaza. This could be set during a time when the sky is in chaos due to some dark energy. Rayquaza is drawn to Ash because of his pure heart and determination. Ash, with his usual courage, teams up with his pokemon to assist Rayquaza in restoring balance. As a result, Rayquaza allows Ash to catch it.
The appeal lies in seeing Ash in new and exciting situations. With legendaries involved, his journey becomes more epic. It's like taking the underdog story of Ash in the anime and supercharging it.
In Ash-centered legendary Pokemon fanfiction, often Ash has extraordinary adventures. He might form unique bonds with legendary Pokemon that are not seen in the official storylines. For example, he could befriend a Mewtwo and together they face off against an evil organization trying to clone more powerful Pokemon. These fanfictions allow for a lot of creativity, expanding on Ash's character and his relationships in the Pokemon world.
Obviously, Ash is one of the main characters. He's the protagonist who has a passion for pokemon and is always eager to become a pokemon master. And the legendary pokemon he encounters or befriends would also be important characters. For instance, if it's Lugia, Lugia would play a major role in the story as it's a very powerful and mysterious pokemon.
Often, Ash has to complete a quest. In a fanfic with Ho - Oh, Ash might have to find three special feathers scattered across the region. These feathers are said to be the key to summoning Ho - Oh. As he embarks on this journey, he faces many challenges and overcomes them with his existing Pokemon team. Once he collects all the feathers, Ho - Oh appears and, impressed by Ash's determination, decides to fight alongside him. Another way is through a prophetic vision. Ash might have a dream that tells him how to find and bond with a Legendary like Entei, and he follows this vision to make it happen.