One possible plotline could be how the Dursleys face magical mishaps in their daily lives that drive them crazy. For example, maybe Dudley accidentally gets turned into a pig by a stray spell and the Dursleys have to deal with that chaos. Another could be that they are constantly haunted by strange magical creatures that are attracted to Harry's presence in their house.
In this fanfic, it might show how the Dursleys' lives become hell when they try to keep Harry's magic a secret from the wizarding world. The magical world could start to interfere in their lives in small ways at first, like their appliances going haywire due to magical interference. Then it could escalate to more serious things like their house being overrun by magical plants that are attracted to Harry. The Dursleys' attempts to keep everything normal would be constantly thwarted, leading to a life of chaos and 'hell' for them.
It might show their fear in a more extreme way. Instead of just being dismissive of magic, they could be absolutely terrified of it. For example, every time Harry does something even slightly magical, they could cower in a corner.
Well, perhaps the arrival of Harry Potter in their lives could be a major factor. His presence might disrupt their normal, mundane existence. They are forced to take care of a wizard child while they are Muggles who seem to despise anything out of the ordinary. His magical outbursts and the constant reminders of the wizarding world that come with him could be making their lives a living hell.
Perhaps in the fanfic, a time - traveling wizard goes back to save Harry from the Dursleys. This would lead to a lot of changes in the timeline. Harry might be introduced to magic much earlier and form different relationships. He could also have a different understanding of his parents' history and his own role in the wizarding world as a result of being removed from the Dursleys' environment.
In certain fanfictions of this type, Harry could be found by a powerful but reclusive wizard. This wizard decides to mentor Harry in the ways of ancient and lost magics. Harry then uses this knowledge to not only become a very powerful wizard but also to change the wizarding world's view on things like blood purity. He may also go on a journey to find out why the Dursleys abandoned him and in the process, uncover some dark secrets about his family that had been long buried.
One possible plotline could be Harry finding a way to secretly practice magic while imprisoned. For example, he might discover a hidden corner in the attic where he can perform small spells without the Dursleys noticing.
In this fanfic, the Dursleys may be depicted as being in over their heads. Vernon Dursley, for example, might be shown as constantly angry and trying to assert his authority in a situation where he has none. Petunia Dursley could be portrayed as being torn between her dislike for magic and her sense of family obligation towards Harry. Dudley might be shown as being bullied or affected in the Muggle world because of Harry's presence in their family.
One possible plotline could be Harry finding a way to break free from the chains and use his magic to confront the Dursleys about their mistreatment. Another could be the Dursleys realizing the error of their ways after chaining Harry up and having a change of heart. Or perhaps there are magical forces at work that lead to a series of adventures while Harry is still chained, like dealing with strange creatures that are attracted to the situation.
One possible plotline could be Harry discovering a hidden magical ability that helps him escape. For example, he might find out he can teleport short distances, which he uses to get away from the Dursleys' house when they are being particularly cruel. Another could be that he gets help from an unexpected magical creature that has been secretly observing him all along. Maybe a house - elf that takes pity on him and shows him a secret passage out of the house.
A great 'Harry Potter Dursleys fanfic' might explore the Dursleys' backstory more deeply. For example, it could show how Vernon's hatred for magic and strange things developed over time. Or it could focus on Petunia's envy of Lily's magical abilities and how that affected her relationship with Harry. Some fanfics also imagine a scenario where the Dursleys are magically transported to Hogwarts and have to adapt to the magical environment. They would be completely out of their element, and it would be interesting to see how they interact with the students and teachers.
One possible plotline could be Harry learning dark magic in Hell but then using it for good in the wizarding world. For example, he might master a powerful spell that can only be learned in Hell to defeat Voldemort once and for all.